Ultrafast transient terahertz conductivity of monolayer MoS₂ and WSe₂ grown by chemical vapor deposition

ACS Nano. 2014 Nov 25;8(11):11147-53. doi: 10.1021/nn5034746. Epub 2014 Nov 4.

Abstract

We have measured ultrafast charge carrier dynamics in monolayers and trilayers of the transition metal dichalcogenides MoS2 and WSe2 using a combination of time-resolved photoluminescence and terahertz spectroscopy. We recorded a photoconductivity and photoluminescence response time of just 350 fs from CVD-grown monolayer MoS2, and 1 ps from trilayer MoS2 and monolayer WSe2. Our results indicate the potential of these materials as high-speed optoelectronic materials.

Keywords: CVD; molybdenum disulfide; photoluminescence; terahertz conductivity; transition metal dichalcogenide; tungsten diselenide; ultrafast.

Publication types

  • Research Support, Non-U.S. Gov't